https://doi.org/10.1007/s100530070039
Number of electrons active in slow collisions of O8+ and Ar8+ with C60
Laboratoire de Spectrométrie Ionique et Moléculaire, Université Lyon 1, Campus de la Doua, 69622 Villeurbanne Cedex, France
Received:
12
November
1999
Revised:
28
February
2000
Published online: 15 October 2000
Electron multiplicity has been measured for collisions of O8+ and Ar8+ with C60
fullerene in coincidence with the number of electrons stabilized on the projectile.
Measurements have been performed at the same velocity v=0.24 a.u. for both systems.
The number of active electrons r is deduced from the number of stabilized electrons s and
the number of ejected electrons n. The kinetic energy spectra of outgoing projectiles are
different for collisions "outside"the C60 cage which show a narrow peak and collisions
"inside"the C60 cage which show a broad shifted energy loss peak. The cross-sections
for stabilization of s electrons have been measured versus
r for each s value
corresponding to peripheral collisions, i.e.
for O8+ and
for Ar8+. Their sum
over s, the total cross-section
, shows a similar behavior for Ar8+ and O8+ up to r=10. It
gives a clear indication of identical multicapture processes for these two systems. The
very different s number distribution is interpreted by the
different relaxation modes of the
multiply excited states of O
and Ar
.
PACS: 36.40.Qv – Stability and fragmentation of clusters / 34.70.+e – Charge transfer
© EDP Sciences, Società Italiana di Fisica, Springer-Verlag, 2000