https://doi.org/10.1007/s100530050178
Electron multiplicity in slow collisions of Ar8+ ions with C60
Laboratoire de Spectrométrie Ionique et Moléculaire (UMR-CNRS 5579) ,
Université Claude Bernard, Lyon I, Bâtiment 207, Campus de la Doua, 69622 Villeurbanne
Cedex, France
Received:
25
March
1998
Accepted:
9
June
1998
Published online: 15 October 1998
Electron capture by Ar8+ in collisions with C60 fullerene has been
investigated using coincident measurements of the number n of ejected
electrons, the mass and charge of multicharged C recoil ions and
their fragments C
and the final charge state of outgoing projectiles
Ar
(
). The number of captured electrons r is the sum of the
numbers of stabilized and emitted electrons: r=n+s. The ratio n/s
decreases by a factor three with s increasing from 1 to 7 showing that the
multiply excited states populated by capture of a large number of electrons
are rather stable against auto-ionisation. Each kinetic energy spectrum of
Ar+ and Ar2+ projectiles is composed of two peaks which we attribute to
collisions "inside" and "outside" the C60 cage. The measured energy shift
of the projectile
keV is consistent with the corresponding energy
loss
keV in a carbon foil with an equivalent thickness. Inside
collisions are characterized by a strong dissociation of recoil ions into
light monocharged fragments and by a high multiplicity of ejected
electrons.
PACS: 36.40.Qv – Stability and fragmentation of clusters / 34.70.+e – Charge transfer
© EDP Sciences, Società Italiana di Fisica, Springer-Verlag, 1998