https://doi.org/10.1140/epjd/s10053-021-00112-9
Regular Article - Clusters and Nanostructures
Submersion of rubidium clusters in helium nanodroplets
1
Institut für Ionenphysik und Angewandte Physik, Universität Innsbruck, Technikerstr. 25, 6020, Innsbruck, Austria
2
Faculté des Sciences IV, Université Libanaise, Haouch El-Omara, Zahlé, Lebanon
Received:
3
November
2020
Accepted:
9
December
2020
Published online:
12
April
2021
Alkali atoms and small clusters are known to reside on the surface of a helium droplet rather than its inside as most other dopant species. A theoretical investigation suggested that alkali clusters (Li–Rb) exceeding a certain critical size can become submerged in the droplet, which was experimentally confirmed for sodium and potassium. Here, we report an analogous experimental study of rubidium cluster submersion by means of electron impact mass spectrometry. We recorded size distributions of Rb cluster ions at various electron energies between 8 and 160 eV. Our data suggest that Rb clusters attached to helium droplets undergo a gradual submersion transition similar to potassium, ultimately leading to the full submersion of clusters larger than atoms. Our findings are consistent with previous theoretical and experimental studies.
Supplementary Information The online version supplementary material available at https://doi.org/10.1140/epjd/s10053-021-00112-9.
© The Author(s) 2021
Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/.