https://doi.org/10.1140/epjd/e2005-00047-3
Laser spectroscopic investigation of Ca atoms in liquid helium
Comparison between spectral properties for liquid helium-3 and helium-4
1
Department of Physics, Toyama University, Gofuku, Toyama 930-8555, Japan
2
Department of Molecular Structure,
Institute for Molecular Science,
Myodaiji, Okazaki 444-8585, Japan
Corresponding author: a moriwaki@sci.toyama-u.ac.jp
Received:
21
September
2004
Revised:
14
March
2005
Published online:
19
April
2005
Excitation and emission spectra of the S0 – P1 and P – S1 transitions of Ca atoms implanted not only in liquid 4He but also in liquid 3He have been measured. It has been found that the excitation spectra for liquid 3He show considerably smaller widths and peak shifts from transition wavelengths of a free Ca atom, in comparison with those for liquid 4He. These spectral characteristics have been well reproduced by our theoretical calculation based on a vibrating bubble model. This calculation has shown that, due to a significant difference in surface tension between the two liquids, the radius of a bubble formed around Ca in liquid 3He is larger than the one in 4He, and that this fact as well as the smaller number density of He atoms in liquid 3He cause weaker perturbation for Ca, resulting in the smaller peak shift and width for liquid 3He.
PACS: 32.30.Jc – Visible and ultraviolet spectra / 36.40.Mr – Spectroscopy and geometrical structure of clusters / 67.40.Yv – Impurities and other defects
© EDP Sciences, Società Italiana di Fisica, Springer-Verlag, 2005